Throughout his life Rev. Chamberlain continued to preach throughout the nation and served in numerous capacities in New York City and elsewhere. He founded the Brooklyn institute of arts and sciences, and was President of the Untied States Evangelical alliance. He was also president and secretary of the American and Foreign Missionary union. He was vice president of the Immigration Committee of the Civic Federation in 1909 and spoke in opposition to further restrictions on immigration, stating that the immigration laws at the time were sufficient to protect the county from undesirable foreigners.
Leander was a resident of Pasadena, California when he died in Altadina on May 9, 1913. He was buried with his wife in Laurel Hill Cemetery in Philadelphia, PA.
Dr. Chamberlain left $63,000 to religious, benevolent and scientific organizations. He also gave $100,000 to an institute in Turkey which he had projected and fostered.
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